Tetrahedral Clustering in Molten Lithium under Pressure

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چکیده

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Tetrahedral clustering in molten lithium under pressure.

A series of electronic and structural transitions are predicted in molten lithium from first principles. A new phase with tetrahedral local order characteristic of sp3 bonded materials and poor electrical conductivity is found at pressures above 150 GPa and temperatures as high as 1000 K. Despite the lack of covalent bonding, weakly bound tetrahedral clusters with finite lifetimes are predicted...

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ژورنال

عنوان ژورنال: Physical Review Letters

سال: 2008

ISSN: 0031-9007,1079-7114

DOI: 10.1103/physrevlett.101.075703